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北京雾霾研究成果在Atmospheric Chemistry and Physics发表，谁分享下啊
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回复此楼» 抢金币啦！回帖就可以得到:
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材料理论模拟或理论计算的作用有多大
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急招科研助理/博士后
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各位大佬帮忙分析一下面上意见，是否上会？几个A、B、C？
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中科院化学所韩布兴院士团队诚聘光催化、光酶催化、光电催化领域博士后1-2名
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山东征女友，坐标济南
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中科院西北研究院招收遥感、地信相关专业联培研究生及科研助理！
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哈工大（深圳）招收工程热物理专业2027入学博士生
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11楼2014-01-27 16:54:36
8楼2014-01-25 10:03:42
9楼2014-01-27 00:32:40
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小木虫: 金币+0.5, 给个红包，谢谢回帖
小木虫: 金币+0.5, 给个红包，谢谢回帖
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Atmos. Chem. Phys., 13, 7053–7074, 2013 www.atmos-chem-phys.net/13/7053/2013/ Chemical characterization and source apportionment of PM2.5 in Beijing: seasonal perspective R. Zhang1,*, J. Jing1,2,*, J. Tao3,*, S.-C. Hsu4,*, G. Wang5, J. Cao5, C. S. L. Lee6, L. Zhu3, Z. Chen7, Y. Zhao7, and Z. Shen8 Abstract. In this study, 121 daily PM2.5 (aerosol particle with aerodynamic diameter less than 2.5 μm) samples were collected from an urban site in Beijing in four months between April 2009 and January 2010 representing the four seasons. The samples were determined for various compositions, including elements, ions, and organic/elemental carbon. Various approaches, such as chemical mass balance, positive matrix factorization (PMF), trajectory clustering, and potential source contribution function (PSCF), were employed for characterizing aerosol speciation, identifying likely sources, and apportioning contributions from each likely source. Our results have shown distinctive seasonality for various aerosol speciations associated with PM2.5 in Beijing. Soil dust waxes in the spring and wanes in the summer. Regarding the secondary aerosol components, inorganic and organic species may behave in different manners. The former preferentially forms in the hot and humid summer via photochemical reactions, although their precursor gases, such as SO2 and NOx, are emitted much more in winter. The latter seems to favorably form in the cold and dry winter. Synoptic meteorological and climate conditions can overwhelm the emission pattern in the formation of secondary aerosols. The PMF model identified six main sources: soil dust, coal combustion, biomass burning, traffic and waste incineration emission, industrial pollution, and secondary inorganic aerosol. Each of these sources has an annual mean contribution of 16, 14, 13, 3, 28, and 26 %, respectively, to PM2.5. However, the relative contributions of these identified sources significantly vary with changing seasons. The results of trajectory clustering and the PSCF method demonstrated that regional sources could be crucial contributors to PM pollution in Beijing. In conclusion, we have unraveled some complex aspects of the pollution sources and formation processes of PM2.5 in Beijing. To our knowledge, this is the first systematic study that comprehensively explores the chemical characterizations and source apportionments of PM2.5 aerosol speciation in Beijing by applying multiple approaches based on a completely seasonal perspective。 |
10楼2014-01-27 10:16:30