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Reviewer #1: The authors described the enhanced photocatalytic efficiency of A@mpg-c3n4 and its application in the detection of PSA. They have performed the detection experiments carefully, but many points have been omitted in the manuscript as mentioned below, which makes the article not suitable for a highly reputed journal like biosensors and bioelectronics. Moreover, the enhanced photocatalytic efficiency of the system has been proved earlier and explained for the degradation of organic dyes. The novel part in the article remains in the use of detection of PSA, hence emphasis may be given to the sensing part. So in my opinion the work will be more suitable for more specific journal.
The authors have given the SEM and TEM image with different magnification. For a comparison the same magnification is needed. Need to give both low and high magnification images to confirm the claimed "sheet like structure of A". To me the structure appears as particles.  Same is the case with all images. SEM of A is not given, why? I would suggest an EDS mapping for the A@mpg-c3n4 to identify the A distribution over mpg-c3n4.
How the carboxyl groups are introduced in the mpg-c3n4? The presence of carboxyl group is not clearly evident in IR? Why such a low intensity for the peak? what is the %of carboxylation?
It appears that the XRD figure caption is wrong. the peak corresponding to mpg-c3n4 is marked in the XRD of A !
What is the wavelength of light used for photoelectrochemical measurements?
X-axis is not given in figure 3A. Experimental condition are also not mentioned. Is it that the light was on for all the time, and added different concentrations of PSA?
What was the concentration of PSA for stability test?


Reviewer #2: Authors have described well technique for the detection of PSA. But there are many early reported sensors which are showing better response. However authors have explained and discussed the results appropriately
Sensors is not optimized in terms of temperature and response time.
All other results are satisfactory explained.


Reviewer #3: The authors should edit the labels in the Fig. 4A regarding the selectivity, to be more correct. for example (b) should be "CEA+PSA", not just "CEA".
The authors should enhance the conclusion part thoroughly. it is not enough.

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