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小木虫论坛-学术科研互动平台» 文献求助区» 检索知识 » 检索知识完结子版 » 求SCI检索证明
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[求助] 求SCI检索证明

题目Au–Pd alloy nanoparticle catalyzed selective oxidation of benzyl
alcohol and tandem synthesis of imines at ambient conditions
作者Wenjing Cui, Qi Xiao, Sarina Sarina
其他Catalysis Today, Volume 235, 15 October 2014, Pages 152-159
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zczcwj: 金币+10, ★★★★★最佳答案 2015-04-21 20:33:21
心静_依然: LS-EPI+1, 感谢应助 2015-04-21 20:45:48
入藏号: WOS:000340946200018
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感谢参与，应助指数 +1
https://apps.webofknowledge.com/ ... age=1&doc=1
Au-Pd alloy nanoparticle catalyzed selective oxidation of benzyl alcohol and tandem synthesis of imines at ambient conditions
作者:Cui, WJ (Cui, Wenjiang)[ 1,2 ] ; Xiao, Q (Xiao, Qi)[ 3 ] ; Sarina, S (Sarina, Sarina)[ 3 ] ; Ao, WL (Ao, Wulan)[ 1 ] ; Xie, MX (Xie, Mengxia)[ 4 ] ; Zhu, HY (Zhu, Huaiyong)[ 3 ] ; Bao, Z (Bao, Zhaorigetu)[ 1 ]


CATALYSIS TODAY


卷: 235
页: 152-159
DOI: 10.1016/j.cattod.2014.04.015

出版年: OCT 15 2014

查看期刊信息

CATALYSIS TODAY  

出版商 ELSEVIER SCIENCE BV, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS

ISSN: 0920-5861
eISSN: 1873-4308

研究领域 Chemistry
Engineering



摘要
Alloy nanoparticles (NPs) of gold and palladium on ZrO2 support (Au-Pd@ZrO2) were found to be highly active in oxidation of benzyl alcohols and can be used for the tandem synthesis of imines from benzyl alcohols and amines via a one-pot, two-step process at mild reaction conditions. The first step of the process is oxidation of benzyl alcohol to benzaldehyde, excellent yields were achieved after 7 h reaction at 40 degrees C without addition of any base. In the second step, aniline was introduced into the reaction system to produced N-benzylideneaniline. The benzaldehyde obtained in the first step was completely consumed within 1 h. A range of benzyl alcohols and amines were investigated for the general applicability of the Au-Pd alloy catalysts. It is found that the performance of the catalysts depends on the Au-Pd metal contents and composition. The optimal catalyst is 3.0 wt% Au-Pd@ZrO2 with a Aud molar ratio 1:1. The alloy NP catalyst exhibited superior catalytic properties to pure AuNP or PdNP because the surface of alloy NPs has higher charge heterogeneity than that of pure metal NPs according to simulation of density function theory (DFT). (C) 2014 Elsevier B.V. All rights reserved.

关键词
作者关键词:Tandem synthesis; Gold and palladium alloy nanoparticles; Benzyl alcohol; Amine; Imine

KeyWords Plus:SUPPORTED GOLD NANOPARTICLES; SOLVENT-FREE OXIDATION; BIMETALLIC CATALYSTS; AEROBIC OXIDATION; MOLECULAR-OXYGEN; PALLADIUM; AMINES; MECHANISM; SIEVES

作者信息
通讯作者地址: Zhu, HY (通讯作者) Queensland Univ Technol, Sch Chem Phys & Mech Engn, Brisbane, Qld 4001, Australia.
  增强组织信息的名称
    Queensland University of Technology  


地址:  [ 1 ] Inner Mongolia Normal Univ, Inner Mongolia Key Lab Green Catalysis, Hohhot 010022, Inner Mongolia, Peoples R China
  增强组织信息的名称
    Inner Mongolia Normal University  
       [ 2 ] Inner Mongolia Vocat Coll Chem Engn, Dept Chem Engn, Hohhot 010070, Inner Mongolia, Peoples R China
[ 3 ] Queensland Univ Technol, Sch Chem Phys & Mech Engn, Brisbane, Qld 4001, Australia
  增强组织信息的名称
    Queensland University of Technology  
[ 4 ] Beijing Normal Univ, Analyt Testing Ctr, Beijing 100875, Peoples R China
  增强组织信息的名称
    Beijing Normal University  


电子邮件地址:hy.zhu@qut.edu.au; zrgt@imnu.edu.cn

基金资助致谢
基金资助机构 授权号
National Natural Science Foundation of China  20966008  
Opening Project of Natural Science Foundation of Inner Mongolia  2010KF02  
Australia Research Council  ARC DP110104990  
查看基金资助信息关闭基金资助信息   

Financial supports from the National Natural Science Foundation of China (No. 20966008), Opening Project of Natural Science Foundation of Inner Mongolia (No. 2010KF02) and Australia Research Council (ARC DP110104990) are gratefully acknowledged.

出版商
ELSEVIER SCIENCE BV, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS

类别 / 分类
研究方向:Chemistry; Engineering

Web of Science 类别:Chemistry, Applied; Chemistry, Physical; Engineering, Chemical

文献信息
文献类型:Article

语种:English

入藏号: WOS:000340946200018

ISSN: 0920-5861

eISSN: 1873-4308

其他信息
IDS 号: AN9RP

Web of Science 核心合集中的 "引用的参考文献": 42

Web of Science 核心合集中的 "被引频次": 2

JCR® 类别 JCR 分区
CHEMISTRY, APPLIED  Q1
CHEMISTRY, PHYSICAL  Q2
ENGINEERING, CHEMICAL  Q1


数据来自第 2013 版 Journal Citation Reports®
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zczcwj

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引用回帖:
3楼: Originally posted by baiyuefei at 2015-04-21 20:25:33
入藏号: WOS:000340946200018

谢谢
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