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The shoulder peak, which is apparently absent in BMBCP, is ascribed to the ICT transition. On one hand, the congested central part where bulky substituents suspend surround the benzene core leads to largely twisted molecular conformation with shortened conjugation, which might result in a blue-shift tendency; on the other hand, the electron-rich TPA units together with the electron-withdrawing –CN induce the ICT effect in the excited state and give rise to red-shifted emission depending on the solvent polarity. The joint effect between the conjugation and ICT degree definesthe emission of DMCS-TPA. |
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