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[资源] Angew. Chem. Int. Ed.最新综述:基于电化学的纳米粒子

Electrochemistry of Nanoparticles 共28页引文357篇
Steven E. F. Kleijn, Stanley C. S. Lai, Marc T. M. Koper,* and Patrick R. Unwin*

S. E. F. Kleijn, Prof. Dr. M. T. M. Koper
Leiden Institute of Chemistry, Leiden University
PO Box 9502, 2300 RA, Leiden (The Netherlands)
E-mail: m.koper@chem.leidenuniv.nl
Dr. S. C. S. Lai, Prof. Dr. P. R. Unwin
Department of Chemistry, University of Warwick
Gibbet Hill Road, Coventry CV4 7AL (UK)
E-mail: p.r.unwin@warwick.ac.uk
Dr. S. C. S. Lai
Current address: MESA+ Institute for Nanotechnology, University of
Twente, PO Box 217, 7500 AE, Enschede (The Netherlands)

M etal nanoparticles (NPs) find widespread application as a result of
their unique physical and chemical properties. NPs have generated
considerable interest in catalysis and electrocatalysis, where they
provide a high surface area to mass ratio and can be tailored to
promote particular reaction pathways. The activity of NPs can be
analyzed especially well using electrochemistry, which probes inter-
facial chemistry directly. In this Review, we discuss key issues related to
the electrochemistry of NPs. We highlight model studies that demon-
strate exceptional control over the NP shape and size, or mass-trans-
port conditions, which can provide key insights into the behavior of
ensembles of NPs. Particular focus is on the challenge of ultimately
measuring reactions at individual NPs, and relating the response to
their structure, which is leading to imaginative experiments that have
an impact on electrochemistry in general as well as broader surface
and colloid science.

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2014-04-11 17:03:05, 3.49 M

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