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Author(s): Chu, Y Y (Chu, Yan-yang); Zhang, D M (Zhang, Dong-mei); Liu, L (Liu, Lei); Qian, Y (Qian,Yi); Li, L L (Li, Ling-ling)
Title: Electrochemical degradation of m-cresol using porous carbon-nanotube-containing cathode and Ti/SnO2-Sb2O5-IrO2 anode: kinetics, byproducts and biodegradability
Source: JOURNAL OF HAZARDOUS MATERIALS, 252-253:306-312 May 2013
ISSN: 0304-3894
DOI: 10.1016/j.jhazmat.2013.03.018

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Electrochemical degradation of m-cresol using porous carbon-nanotube-containing cathode and Ti/SnO2-Sb2O5-IrO2 anode: Kinetics, byproducts and biodegradability
作者: Chu, YY (Chu, Yanyang)[ 1 ] ; Zhang, DM (Zhang, Dongmei)[ 1 ] ; Liu, L (Liu, Lei)[ 1 ] ; Qian, Y (Qian, Yi)[ 1 ] ; Li, LL (Li, Lingling)[ 1 ]
来源出版物: JOURNAL OF HAZARDOUS MATERIALS  卷: 252 页: 306-312 DOI: 10.1016/j.jhazmat.2013.03.018 出版年: MAY 15 2013
被引频次: 1 (来自 Web of Science)
引用的参考文献: 36    [ 查看 Related Records ]    引证关系图引证关系图
摘要: The degradation of m-cresol solution was studied using an electrochemical oxidation system with Ti/SnO2-Sb2O5-IrO2 anode for anodic oxidation and porous carbon-nanotube-containing cathode for H2O2 electrogeneration along with Fe3+ reduction. Organic pollutants were oxidized by hydroxyl radical ((OH)-O-center dot) formed simultaneously in the medium from electro-Fenton reaction in the presence of Fe2+ and at the anode surface from water oxidation. The porous cathode made of graphite, carbon nanotube (CNT) and polytetrafluoroethene (PIPE) exhibited a higher catalytic activity toward O-2 reduction producing H2O2 and Fe3+ reduction for Fe2+ regeneration, favoring organics degradation by electro-Fenton oxidation. The degradation kinetics results revealed that the reaction of m-cresol cleavage with hydroxyl radicals could be described by pseudo first-order kinetics. The progress of organics mineralization demonstrated some byproducts were formed during m-cresol degradation. Based on the byproducts identified by GC-MS and HPLC, the sequential process of m-cresol degradation was proposed. Furthermore, the aerobic biological treatment showed that the electrochemical treatment was able to evidently enhance the biodegradability of m-cresol solution. (c) 2013 Elsevier B.V. All rights reserved.
入藏号: WOS:000320288800037
文献类型: Article
语种: English
作者关键词: Electro-Fenton; Degradation; m-Cresol; Carbon nanotube; Byproducts; Biodegradability
KeyWords Plus: BORON-DOPED DIAMOND; ADVANCED OXIDATION PROCESSES; ELECTRO-FENTON DEGRADATION; FELT CATHODE; WASTE-WATER; HYDROGEN-PEROXIDE; AQUEOUS-MEDIUM; DYE; MINERALIZATION; PHENOL
通讯作者地址: Chu, YY (通讯作者) Qingdao Univ Sci & Technol, Sch Environm & Safety Engn, Qingdao 266042, Shandong, Peoples R China.
  增强组织信息的名称
Qingdao University of Science & Technology

地址:  [ 1 ] Qingdao Univ Sci & Technol, Sch Environm & Safety Engn, Qingdao 266042, Shandong, Peoples R China
  增强组织信息的名称
Qingdao University of Science & Technology

电子邮件地址: cyyf200611@qust.edu.cn
基金资助致谢:
基金资助机构授权号
National Natural Science Foundation of China  50808103

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This research was funded by National Natural Science Foundation of China under grant no. 50808103.

出版商: ELSEVIER SCIENCE BV, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
Web of Science 类别: Engineering, Environmental; Engineering, Civil; Environmental Sciences
研究方向: Engineering; Environmental Sciences & Ecology
IDS 号: 162TL
ISSN: 0304-3894