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1¡¢In the inflection discussion, the authors may wish to add that the deviation for high-limit Arrhenius behavior denotes the "effective" rheological wax appearance temperature. 2¡¢We feel that there could very well be subtle mass balance effects here where the silica is effectively sequestering the heavy polars from the bulk fluid (via adsorption), and reducing the nucleation effect of the polar components, while also simultaneously "covering up" themselves with heavy polars, negating the nucleation effects of the inherent SiO2. This could be a very interesting interplay, but the authors must in the final analysis decide how they wish to interpret the data. (Of course the opposite effect is paradoxically observed in the rheology..) ÕâÁ½¸öÎÊÌâÎÒÓе㿴²»¶®£¬Çë´ó¼Ò°ïÎÒ¿´Ò»ÏÂʲôÒâ˼£¬¸ÃÔõô»Ø´ð£¿ 3¡¢The crystallization process can be influenced by the particular choice of cooling rate (5¡ãC/min). How sensitive to this choice were the reported WAT ́s? Moreover, the cooling rate for the microscopy experiments was also 5¡ãC/min, however the rheological measurements were carried out at a cooling rate of 0.5 ¡ãC/min. Please clarify and justify the choice of cooling rate. ÆäʵÎÒÒ²²»ÖªµÀΪʲôѽ£¬ÒòΪÎÒ¿´´ó¼ÒµÄÂÛÎͼÊÇÕâô×öµÄ£¬µ«ÊÇÎÒ¸ÃÔõô»Ø¸´Éó¸åÈ˵ÄÎÊÌâÄØ£¿ ÔÚÏß¼±µÈ |
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1¡¢In the inflection discussion, the authors may wish to add that the deviation for high-limit Arrhenius behavior denotes the "effective" rheological wax appearance temperature. ÔÚ¹Õµã·ÖÎöÖÐ×÷Õß¿ÉÄÜÏ£Íû²¹³ä°¢Â×ÄáÎÚ˹behaviorµÄÎó²î¶ÔÁ÷Ìå̬ÎöÀ¯µãµÄÓ°Ïì¡£ 2¡¢We feel that there could very well be subtle mass balance effects here where the silica is effectively sequestering the heavy polars from the bulk fluid (via adsorption), and reducing the nucleation effect of the polar components, while also simultaneously "covering up" themselves with heavy polars, negating the nucleation effects of the inherent SiO2. This could be a very interesting interplay, but the authors must in the final analysis decide how they wish to interpret the data. (Of course the opposite effect is paradoxically observed in the rheology..) ÎÒÃÇÈÏΪÖÊÁ¿Æ½ºâµÄÓ°ÏìÔÚ±¾´ÎÊÔÑéÖÐ΢ºõÆä΢£¬¹èÔ×Ó´ÓÌå»ýÁ÷ÌåÖÐÓÐЧµØ¸ôÀëÁËÖØÖʼ«ÐÔÎïÖÊ£¬¼õСÁ˼«ÐÔ×é·Ö³ÉºËЧӦ£¬µ«ÊÇÒ²ÓÃÖØ×é·ÖµÄ¼«ÐÔ¸²¸Ç×ÔÉí£¬ºöÂÔÁ˶þÑõ»¯¹è±¾ÉíµÄ³ÉºËЧӦ¡£ÕâÊÇÒ»¸ö·Ç³£ÓÐÒâ˼µÄÏ໥ӰÏì×÷Ó㬵«ÊÇ×÷Õß±ØÐëÔÚ×îºóµÄ·ÖÎöÀï¾ö¶¨ÈçºÎ½âÊÍÕâЩÊý¾Ý¡£ ¼ûµ½Ó¢ÎÄÎÄÏ×¾ÍÏñ·ÒëÏ£¬ |
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