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叶金花携昔日弟子唐军旺在Chem. Soc. Rev发表的Ag3PO4光催化综述
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伦敦学院的唐军旺教授最近几年在jacs，angew，ees上发表了几篇重量级的光催化研究论文，随后在ees写了一篇光催化综述（详情可见http://muchong.com/bbs/viewthread.php?tid=8413503），现又与其早年博导叶金花教授（磷酸银光催化的鼻祖）一起在Chem. Soc. Rev.上对火热的磷酸银光催化做了一个全面的综述和回顾，题目为Efficient visible driven photocatalyst, silver phosphate: performance, understanding and perspective，共21页，参考文献82篇。 光催化技术非常有前途，因为它可以产生可再生能源和治理水污染。为了能够让这个技术推入实际应用，发展高效的可见光催化剂是非常有必要的，比如磷酸银。这篇综述文章旨在于突出磷酸银的一些最新研究进展，主要聚焦于其在产氧，有机污染物降解的光催化应用。 期刊： Chem. Soc. Rev., 2015, Advance Article DOI: 10.1039/C5CS00380F Received 11 May 2015, First published online 23 Jul 2015 题目： Efficient visible driven photocatalyst, silver phosphate: performance, understanding and perspective 作者： David James Martin,abc Guigao Liu,de Savio J. A. Moniz,a Yingpu Bi,f Andrew M. Beale,bc Jinhua Ye*degh and Junwang Tang*a 摘要： Photocatalysis is a promising technology that can contribute to renewable energy production from water and water purification. In order to further develop the field and meet industrial requirements, it is imperative to focus on advancing high efficiency visible light photocatalysts, such as silver phosphate (Ag3PO4). This review aims to highlight the recent progress made in the field, focusing on oxygen production from water, and organic contaminant decomposition using Ag3PO4. The most important advances are discussed and explained in detail, including semiconductor–semiconductor junctions, metal–semiconductor junctions, exposing facet control, and fundamental understanding using advanced spectroscopies and computational chemistry. The review then concludes by critically summarising both findings and current perspectives, and ultimately how the field might best advance in the near future.  1.jpg [ Last edited by 罗马里奥 on 2015-7-24 at 21:13 ] |
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对于该方向零基础，纯粹了解了解，看到一句话不是很明白，想请楼主指点指点：Ag3PO4 possesses a very deep valence band, located approximately +2.9 V vs. NHE (Normal Hydrogen Electrode, pH 0), and therefore is well aligned for oxidation reactions. However, the conduction band is located at +0.45 V vs. NHE (pH 0), meaning that H+ cannot be reduced to H2 fuel, and thus the compound cannot be used for overall water splitting.是什么意思啊？为什么空带和导带都是正的呢？不是应该一个在0之上，一个在0之下吗？为什么说相应的数值就能氧化水不能还原得到氢呢？ |
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2015-07-24 10:13
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