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5Â¥2008-06-23 23:23:01
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2Â¥2008-06-23 19:45:28
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Article abstract -------------------------------------------------------------------------------- Nature Materials Published online: 22 June 2008 | doi:10.1038/nmat2219 Direct observation of a local structural mechanism for dynamic arrest C. Patrick Royall1,2, Stephen R. Williams3, Takehiro Ohtsuka2 & Hajime Tanaka2 -------------------------------------------------------------------------------- AbstractThe mechanism by which a liquid may become arrested, forming a glass or gel, is a long-standing problem of materials science. In particular, long-lived (energetically) locally favoured structures (LFSs), the geometry of which may prevent the system relaxing to its equilibrium state, have long been thought to play a key role in dynamical arrest. Here, we propose a definition of LFSs which we identify with a novel topological method and directly measure with experiments on a colloidal liquid¨Cgel transition. The population of LFSs is a strong function of (effective) temperature in the ergodic liquid phase, rising sharply approaching dynamical arrest, and indeed forms a percolating network that becomes the 'arms' of the gel. Owing to the LFSs, the gel is unable to reach equilibrium, crystal¨Cgas coexistence. Our results provide direct experimental observation of a link between local structure and dynamical arrest, and open a new perspective on a wide range of metastable materials. |
3Â¥2008-06-23 23:17:01
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4Â¥2008-06-23 23:21:48













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