| ²é¿´: 4699 | »Ø¸´: 103 | ||||||||
| ¡¾½±Àø¡¿ ±¾Ìû±»ÆÀ¼Û96´Î£¬×÷Õßdenny_kennyÔö¼Ó½ð±Ò 75.2 ¸ö | ||||||||
| µ±Ç°Ö»ÏÔʾÂú×ãÖ¸¶¨Ìõ¼þµÄ»ØÌû£¬µã»÷ÕâÀï²é¿´±¾»°ÌâµÄËùÓлØÌû | ||||||||
[×ÊÔ´]
Chemical review ×îйâºÏ³É´ß»¯µÄ´ó×÷
|
||||||||
|
Table of Contents 1. Introduction 1.1. The Oxygen Evolving Complex ¨C The Site Where Water Is Oxidized 1.2. Artificial Photosynthesis ¨C Architectural Complexity 1.2.1. Light Absorption by a Chromophore ¨C The Photosensitizer 1.2.2. Reduction of Protons for the Generation of Solar Fuels ¨C The Reduction Catalyst 1.2.3. The Water Oxidation Catalyst ¨C Catalytic Complexity at the Frontier 1.3. Experimental Design for Evaluating Water Oxidation Catalysts 1.3.1. Commonly Used Chemical Oxidants 1.3.2. Light-Driven Water Oxidation 1.3.3. (Photo)electrochemical Water Oxidation 1.3.4. Homogeneous versus Heterogeneous Catalysis ¨C The Conversion of Molecular Entities to Heterogeneous Catalytically Active Species 1.4. Mechanistic Considerations Associated with Artifical Water Oxidation Catalysts 2. Molecular Ruthenium-Based Water Oxidation Catalysts 2.1. Dinuclear Ruthenium-Based Systems for Water Oxidation 2.2. Single-Site Ruthenium-Based Catalysts ¨C Simple and Efficient 2.2.1. Mononuclear Ruthenium Catalysts Comprising Neutral Ligand Frameworks 2.2.2. Mononuclear Ruthenium Catalysts Containing Anionic Ligand Backbones 3. Iridium-Based Systems for Water Oxidation 3.1. Cyclometalated Iridium Complexes 3.2. Iridium Catalysts Based on Cyclopentadiene-Type Ligands 3.3. Development of Iridium N-Heterocyclic Carbene and Other Iridium Catalysts 3.4. Decomposition of Homogeneous Iridium Catalysts ¨C Generation of Catalytically Active Heterogeneous Iridum Species 4. Artificial Catalysts Housing Earth-Abundant First-Row Transition Metals 4.1. Early Biomimetic Manganese-Based Photosynthetic Mimics 4.2. Manganese-Based Catalysts Capable of Generating Oxygen 4.3. Molecular Water Oxidation Catalysts Based on Iron 4.4. Oxygen Formation in Copper-Based Systems 4.5. Cobalt-Based Catalysts Capable of Oxidizing Water 5. Synthetic Metal¨COxo Mimics of the Oxygen Evolving Complex 5.1. Polyoxometalates ¨C The Molecular, Inorganic Alternative 5.1.1. Ruthenium-Based Polyoxometalates 5.1.2. Cobalt-Based Polyoxometalates ¨C The Ambiguity of Distinguishing between Homogeneous and Heterogeneous Catalysis 5.1.3. Other Metal-Based Polyoxometalates 5.2. Metal Cubanes Based on Earth-Abundant Metals as Water Oxidation Catalysts 5.2.1. The Self-Assembling Cobalt¨CPhosphate (Co¨CPi) Catalyst 5.2.2. Cobalt Cubanes and Related Cobalt Oxide Materials as Oxygen Evolving Catalysts 5.2.3. Manganese Cubanes as Water Oxidation Catalysts 6. Conclusions |
» ±¾Ìû¸½¼þ×ÊÔ´Áбí
-
»¶Ó¼à¶½ºÍ·´À¡£ºÐ¡Ä¾³æ½öÌṩ½»Á÷ƽ̨£¬²»¶Ô¸ÃÄÚÈݸºÔð¡£
±¾ÄÚÈÝÓÉÓû§×ÔÖ÷·¢²¼£¬Èç¹ûÆäÄÚÈÝÉæ¼°µ½ÖªÊ¶²úȨÎÊÌ⣬ÆäÔðÈÎÔÚÓÚÓû§±¾ÈË£¬Èç¶Ô°æÈ¨ÓÐÒìÒ飬ÇëÁªÏµÓÊÏ䣺xiaomuchong@tal.com - ¸½¼þ 1 : Artificial_Photosynthesis_Molecular_Systems_for_Catalytic_Water_Oxidation.pdf
2014-10-30 17:23:03, 7.05 M
» ÊÕ¼±¾ÌûµÄÌÔÌûר¼ÍƼö
²ÄÁÏÎïÀíÓ뻯ѧ | ÎÄÏ× | ʵÑé·ÖÎö·½·¨ | ¹â´ß»¯²ÄÁÏ |
ÓлúºÏ³É | Ç°ÑØÂÛÎÄ |
» ²ÂÄãϲ»¶
ºþ±±Ê¦·¶´óѧ¸´ÊÔµ÷¼Á
ÒѾÓÐ0È˻ظ´
Î人·ÄÖ¯´óѧ_»¯¹¤Ñ§Ôº¹Ù·½µ÷¼ÁȺ-ԺʿÍŶÓÕÐÉú-ѧÉú×ÔÓɶȸß-ÿ½ì·¢Õ¹ºÃ
ÒѾÓÐ0È˻ظ´
ÎÞ»ú»¯Ñ§ÂÛÎÄÈóÉ«/·ÒëÔõôÊÕ·Ñ?
ÒѾÓÐ233È˻ظ´
¼ÃÄÏ´óѧ¹ú¼ÒÓÅÇà¿ÎÌâ×é 2026 µ÷¼ÁÕÐÉúÀ´À²
ÒѾÓÐ0È˻ظ´
Î人·ÄÖ¯´óѧ_»¯Ñ§Ôº¹Ù·½µ÷¼ÁȺ-ԺʿÍŶÓÕÐÉú-ѧÉú×ÔÓɶȸ߷¢Õ¹ºÃ-»¶Ó¸÷λͬѧ
ÒѾÓÐ0È˻ظ´
Î÷»ª´óѧ »¯Ñ§ µ÷¼ÁÓÐÃû¶î
ÒѾÓÐ0È˻ظ´
ÉϺ£Ó¦Óü¼Êõ´óѧÕÐÉúµ÷¼ÁÑо¿Éú
ÒѾÓÐ7È˻ظ´
» ±¾Ö÷ÌâÏà¹Ø¼ÛÖµÌùÍÆ¼ö£¬¶ÔÄúͬÑùÓаïÖú:
Chemical Review¶þÑõ»¯îÑר¿¯
ÒѾÓÐ374È˻ظ´
ËÕµ³ÉúÀÏʦ ×îРchemical review
ÒѾÓÐ13È˻ظ´
×îÐÂChemical Society Review--Ïß×´Ì«ÑôÄÜµç³Ø
ÒѾÓÐ112È˻ظ´
Chemical Reviews×îÐÂ×ÛÊö£ºÒìÏàÄÉÃ׸´ºÏÎï´ß»¯¼ÁÖеĴ߻¯Ðͬ×÷ÓÃ
ÒѾÓÐ36È˻ظ´
¹úÄÚ¹â´ß»¯¿ÎÌâ×é×îÐÂReveiwÒ»ÀÀ£¨ÒѸ½²¿·ÖPDF¹©ÏÂÔØ£©
ÒѾÓÐ211È˻ظ´
chemical review 2012Äê×î½üµÄCore/Shell NanoparticlesµÄ×ÛÊö
ÒѾÓÐ42È˻ظ´
Chemical ReviewÉÏÃæ×îÐµĹØÓÚMOFsµÄÎÄÕÂ
ÒѾÓÐ85È˻ظ´
lh121961
ÖÁ×ðľ³æ (ÖªÃû×÷¼Ò)
- Ó¦Öú: 25 (СѧÉú)
- ½ð±Ò: 15280.2
- Ìû×Ó: 6184
- ÔÚÏß: 8552.9Сʱ
- ³æºÅ: 2077032
3Â¥2014-10-30 19:23:11
¼òµ¥»Ø¸´
8dianbao2Â¥
2014-10-30 17:51
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
weizhen7114Â¥
2014-10-31 00:21
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
chemmatworm5Â¥
2014-10-31 05:22
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
zjjxl6Â¥
2014-10-31 06:50
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
wjy20117Â¥
2014-10-31 08:56
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
ccsclver20088Â¥
2014-10-31 09:06
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
sheriden20069Â¥
2014-10-31 10:35
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
nanofeifei10Â¥
2014-10-31 11:08
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
ÈôÖ»Èç³õjian11Â¥
2014-10-31 11:18
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
ÌìÌ÷½Ïò12Â¥
2014-10-31 11:44
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
ǧèó13Â¥
2014-10-31 12:02
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
62693948514Â¥
2014-10-31 13:29
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡













»Ø¸´´ËÂ¥
5