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书名Metal Nanoparticles for Catalysis Advances and Applications 作者Franklin Tao University of Notre Dame, USA Email: franklin.tao.2011@gmail.com 页数284 出版社 RSC PRESS Print ISBN: 978-1-78262-033-4 PDF eISBN: 978-1-78262-103-4 Chapter 1 Introduction: Synthesis and Catalysis on Metal Nanoparticles 1 Franklin (Feng) Tao, Luan Nguyen and Shiran Zhang Chapter 2 Nanocatalysis: Definition and Case Studies 6 Choumini Balasanthiran and James D. Hoefelmeyer 2.1 Introduction 6 2.1.1 Flash Synopsis of the History of Catalysis 7 2.1.2 Reporting Turnover Frequency: the Common Denominator in Catalysis 8 2.2 Factors Contributing to Structure Sensitivity in Catalysis 9 2.2.1 Statistical Shape Analysis of Polyhedra Crystals and Relation to Catalysis 9 2.2.2 Equilibrium Shapes of Nanocrystals 11 2.2.3 Surface Restructuring 12 2.2.4 Mobility of Surface Adsorbates 14 2.2.5 Change in the Electronic Structure of Solids at the Nanometre Scale 14 2.2.6 Example to Illustrate Anomalous TOF Behavior: Ethane Hydrogenolysis on Rhodium 15 2.3 Synthesis and Properties of Well-defined Nanocrystals 16 2.4 The Dawn of Nanocatalysis and Case Studies 18 2.4.1 CO Oxidation on Au 18 2.4.2 TiO2 Nanocrystals with Reactive Facets 19 2.4.3 Catalysis on Shape-controlled Pt Nanocrystals 21 RSC Catalysis Series No. 17 Metal Nanoparticles for Catalysis: Advances and Applications Edited by Franklin Tao r The Royal Society of Chemistry 2014 Published by the Royal Society of Chemistry, www.rsc.org ix . Published on 12 June 2014 on http://pubs.rsc.org | doi:10.1039/9781782621034-FP009 2.4.4 Advanced Templating Methods for Nanocrystal Synthesis 23 2.4.5 Hybrid Nanocrystal Catalysis 23 2.5 Conclusion 24 References 25 Chapter 3 New Strategies to Fabricate Nanostructured Colloidal and Supported Metal Nanoparticles and their Efficient Catalytic Applications 30 Kohsuke Mori and Hiromi Yamashita 3.1 Introduction 30 3.2 New Route for the Preparation of Supported Metal Nanoparticle Catalysts 31 3.2.1 A Photo-assisted Deposition Method Using a Single-site Photocatalyst 31 3.2.2 A Microwave-assisted Deposition Method 34 3.2.3 Deposition of Size-controlled Metal Nanoparticles as Colloidal Precursors 35 3.3 Multifunctional Catalysts Based on Magnetic Nanoparticles 38 3.3.1 Core–shell Magnetic FePt@Ti-containing Silica Spherical Nanocatalyst 38 3.3.2 Water-soluble FePt Magnetic NPs Modified with Cyclodextrin 39 3.3.3 FePd Magnetic NPs Modified with a Chiral BINAP Ligand 41 3.3.4 Core–shell Nanostructured Catalyst for One-pot Reactions 42 References 44 Chapter 4 Organometallic Approach for the Synthesis of Noble Metal Nanoparticles: Towards Application in Colloidal and Supported Nanocatalysis 47 Solen Kinayyigit and Karine Philippot 4.1 Introduction 47 4.2 Organometallic Synthesis of Noble Metal Nanoparticles 48 4.3 Nanoparticles for Colloidal Catalysis 49 4.3.1 Hydrogenation Reactions 50 4.3.1.1 Ligand Stabilized Nanoparticles as Catalysts 50 4.3.1.2 Water-soluble Nanoparticles as Catalysts 52 x Contents . Published on 12 June 2014 on http://pubs.rsc.org | doi:10.1039/9781782621034-FP009 View Online  QQ截图20140724202011.png |
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