| ²é¿´: 2151 | »Ø¸´: 26 | |||||||
| ¡¾½±Àø¡¿ ±¾Ìû±»ÆÀ¼Û26´Î£¬×÷Õßnowitzki_ciÔö¼Ó½ð±Ò 19.8 ¸ö | |||||||
nowitzki_ciר¼Ò¹ËÎÊ (ÖøÃûдÊÖ)
|
[×ÊÔ´]
Phys. Chem. Chem. Phys.Èȵã×ÛÊö£ºµ±ºê¹ÛÓöµ½Î¢¹Û
|
||||||
|
This article is part of themed collection: PCCP¡¯s 15th anniversary Where macro meets micro ¹²13Ò³ ÒýÎÄ73ƪ ÇëС»ï°éÃÇÏÂÔØºó¸ø¸öºÃÆÀ£¡ R. Stephen Berry*a and Boris M. Smirnov b a The University of Chicago, 929 East 57th Street, Chicago, Illinois, USA. E-mail: berry@uchicago.edu; Tel: +1 773 702 7021 b Joint Institute for High Temperatures, RAN 13/19, Moscow 125412, Russia DOI: 10.1039/c3cp54550d Reconciling or somehow linking the macroscopic and microscopic approaches to chemical and physical processes has been a challenge unaddressed for many years. One approach, presented here, treats the issue by examining individual phenomena well described by a macro approach that fails when applied to small systems. The key to the approach is determining the approximate system size below which the breakdown of the macro description is observable. The most developed example is the failure of the Gibbs phase rule for sufficiently small atomic clusters. Other examples, such as the onset, at sufficient size, of the insulator-to-metal transition, are discussed, as are some still more challenging phenomena. |
» ±¾Ìû¸½¼þ×ÊÔ´Áбí
-
»¶Ó¼à¶½ºÍ·´À¡£ºÐ¡Ä¾³æ½öÌṩ½»Á÷ƽ̨£¬²»¶Ô¸ÃÄÚÈݸºÔð¡£
±¾ÄÚÈÝÓÉÓû§×ÔÖ÷·¢²¼£¬Èç¹ûÆäÄÚÈÝÉæ¼°µ½ÖªÊ¶²úȨÎÊÌ⣬ÆäÔðÈÎÔÚÓÚÓû§±¾ÈË£¬Èç¶Ô°æÈ¨ÓÐÒìÒ飬ÇëÁªÏµÓÊÏ䣺xiaomuchong@tal.com - ¸½¼þ 1 : c3cp54550d.pdf
2014-05-21 11:39:13, 1.71 M
» ÊÕ¼±¾ÌûµÄÌÔÌûר¼ÍƼö
Nano&Micro | ¿ÆÑа¡ ŬÁ¦°¡ Ï£ÍûÓÐÓð¡ | Nano Self-Assembly |
» ²ÂÄãϲ»¶
¼ÃÄÏ´óѧ¹ú¼ÒÓÅÇà¿ÎÌâ×é 2026 µ÷¼ÁÕÐÉúÀ´À²
ÒѾÓÐ0È˻ظ´
Î人·ÄÖ¯´óѧ_»¯Ñ§Ôº¹Ù·½µ÷¼ÁȺ-ԺʿÍŶÓÕÐÉú-ѧÉú×ÔÓɶȸ߷¢Õ¹ºÃ-»¶Ó¸÷λͬѧ
ÒѾÓÐ0È˻ظ´
ÎÞ»ú»¯Ñ§ÂÛÎÄÈóÉ«/·ÒëÔõôÊÕ·Ñ?
ÒѾÓÐ216È˻ظ´
Î÷»ª´óѧ »¯Ñ§ µ÷¼ÁÓÐÃû¶î
ÒѾÓÐ0È˻ظ´
ÉϺ£Ó¦Óü¼Êõ´óѧÕÐÉúµ÷¼ÁÑо¿Éú
ÒѾÓÐ7È˻ظ´
ÄϾ©ÏþׯѧԺÂÌÉ«ÄÜÔ´²ÄÁÏÍŶÓÕÐÉú
ÒѾÓÐ0È˻ظ´
ÄϾ©ÏþׯѧԺÂÌÉ«ÄÜÔ´²ÄÁÏÍŶÓÕÐÉú
ÒѾÓÐ0È˻ظ´
» ±¾Ö÷ÌâÏà¹Ø¼ÛÖµÌùÍÆ¼ö£¬¶ÔÄúͬÑùÓаïÖú:
ÎÄÕ±»polymer¾Ü¸å£¬ÏëͶJ. Phys. Chem. B£¬²»ÖªµÀÐв»ÐС£
ÒѾÓÐ13È˻ظ´
ѰÕÒ Chem Phys Chem ÔÓÖ¾
ÒѾÓÐ4È˻ظ´
´¿ÎïÀíÀ࣬ÏëͶµ½J. Chem. Phys.ÇëÎÊ¿ÉÒÔÂ𣿻¹ÊDZØÐëÒªºÍ»¯Ñ§ÓÐһЩÁªÏµ£¿
ÒѾÓÐ11È˻ظ´
J. Phys. D: Appl. PhysÓëJAP±È½ÏÄĸö±È½ÏºÃÒ»µã
ÒѾÓÐ23È˻ظ´
¼±ÇóJ Phys Chem LettÔÚEndnoteÀïµÄÎÄÏ׸ñʽ
ÒѾÓÐ3È˻ظ´
ͶJ Phys Chem Lett»¹ÊÇAnal Chem£¿
ÒѾÓÐ21È˻ظ´
J. Phys. Chem. BµÄÎÄÕÂ×ÖÌåͼƬ¸ñʽҪÇóÊÇʲô£¿£¿£¿£¿
ÒѾÓÐ4È˻ظ´
J. Phys. Chem. C½ÓÊÕ£¬·¢ÌùÇì×£Ò»ÏÂ!
ÒѾÓÐ42È˻ظ´
Çë¸ßÊÖÖ¸½Ìһϣ¬INT J QUANTUM CHEMºÍJ PHYS ORG CHEMÕâÁ½±¾ÔÓÖ¾ÔõôÑù£¿
ÒѾÓÐ7È˻ظ´
Macromol. Chem. Phys.ÓÐûÓÐproof?
ÒѾÓÐ5È˻ظ´
Ͷ¸åJ Phys Chem LettÓëChem Mater£¬Ñ¡ÔñÄĸöÄØ£¿
ÒѾÓÐ3È˻ظ´
Mater.Chem. Phys.
ÒѾÓÐ4È˻ظ´
±»J.Phys.Chem C¾ÜÁË£¬2¸öÉó¸åÈËÒâ¼û²î±ðºÜ´ó£¬Óöµ½ÕâÖÖÇé¿öÎÒ¸ÃÕ¦°ì
ÒѾÓÐ16È˻ظ´
J. Phys. Chem. AͶ¸åÇóÖú£¡
ÒѾÓÐ14È˻ظ´
J. Phys. Chem. A,B,C ÕâÈý¸öÔÓÖ¾Äĸö±È½ÏÅ££¿
ÒѾÓÐ17È˻ظ´
chem.phys.lett ÊôÓÚÄĸöÊý¾Ý¿â
ÒѾÓÐ6È˻ظ´
ÇëÎÊJ Phys Chem CÊǼ¸ÇøÆÚ¿¯£¿
ÒѾÓÐ7È˻ظ´
¡¾Óн±»î¶¯¡¿¹ØÓÚJ.Phys.Chem.LetterµÄÊՏ寫ºÃ
ÒѾÓÐ6È˻ظ´
¼òµ¥»Ø¸´
ÁÖ×Ï2Â¥
2014-05-21 18:07
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
JohnÁú3Â¥
2014-05-21 19:15
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
bailang4444Â¥
2014-05-22 20:17
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
waiwaide5Â¥
2014-05-23 08:44
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
zhulw6Â¥
2014-05-23 08:53
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
lanxzh7Â¥
2014-05-23 09:19
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
zhanglexi8Â¥
2014-05-23 10:54
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
s2006210409Â¥
2014-05-23 20:10
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
wjy201110Â¥
2014-05-24 08:05
»Ø¸´
Ò»°ã ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
yuan99911Â¥
2014-05-24 15:37
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
feynmanka12Â¥
2014-05-25 10:51
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
´óË®±13Â¥
2014-05-25 12:29
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
shiyunbuji14Â¥
2014-05-25 16:25
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
ÇåÖ®Òô15Â¥
2014-05-27 23:01
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
Hanbingwf16Â¥
2014-05-28 05:42
»Ø¸´
ÈýÐÇºÃÆÀ
liuhuizhao17Â¥
2014-05-28 08:08
»Ø¸´
ÈýÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
wjwang12318Â¥
2014-05-28 08:52
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
fire2hell19Â¥
2014-05-28 09:51
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
cqu355520Â¥
2014-05-28 11:35
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
chemphys21Â¥
2014-05-28 11:57
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
doveyu22Â¥
2014-05-30 07:00
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
shengmao23Â¥
2014-05-31 10:07
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
SCIxiang24Â¥
2014-09-19 21:02
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
duguqiuxue25Â¥
2015-04-16 23:07
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
haxixi26Â¥
2015-04-17 11:50
»Ø¸´
ÎåÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡
weilucq27Â¥
2015-09-25 20:04
»Ø¸´
ÈýÐÇºÃÆÀ ¶¥Ò»Ï£¬¸Ðл·ÖÏí£¡














»Ø¸´´ËÂ¥