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[资源] 【剑桥新书】Polymer Physics: Applications to ... Thermoreversible Gelation

Polymer Physics: Applications to Molecular Association and Thermoreversible Gelation
Fumihiko Tanaka (Kyoto University, Japan)
Publisher: Cambridge University Press
Publication Date: May 16, 2011
Format: PDF；File Size: 3.66MB；Page: 405
ISBN 978-0-521-86429-9

The field of polymer science has advanced and expanded considerably in recent years, encompassing broader ranges of materials and applications. In this book, Fumihiko Tanaka unifies the subject matter, pulling together research to provide an updated and systematic presentation of polymer association and thermoreversible gelation, one of the most rapidly developing areas in polymer science. Starting with a clear exposition of the fundamental laws of polymer physics, subsequent chapters discuss a new theoretical model that combines thermodynamic and rheological theory. Recent developments in polymer physics are explored, along with important case studies on topics such as self-assembly, supramolecules, thermoreversible gels and water-soluble polymers. Throughout the book, a balance is maintained between theoretical descriptions and practical applications, helping the reader to understand complex physical phenomena and their relevance in industry. This book has wide interdisciplinary appeal and is aimed at students and researchers in physics, chemistry and materials science.[ Last edited by 中山羊 on 2012-3-6 at 14:23 ]

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2012-03-06 14:16:46, 3.66 M

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Contents
Preface page xiii
1 Statistical properties of polymer chains 1
1.1 Conformation of polymers 1
1.2 The ideal chain 5
1.3 Fundamental properties of a Gaussian chain 11
1.4 Effect of internal rotation and stiff chains 13
1.5 Excluded-volume effect 16
1.6 Scaling laws and the temperature blob model 19
1.7 Coil–globule transition of a polymer chain in a poor solvent 21
1.8 Coil–helix transition 23
1.9 Hydration of polymer chains 33
References 44
2 Polymer solutions 46
2.1 Thermodynamics of phase equilibria 46
2.2 Characteristic properties of polymer solutions 57
2.3 Lattice theory of polymer solutions 69
2.4 Scaling laws of polymer solutions 87
References 95
3 Classical theory of gelation 97
3.1 What is a gel? 97
3.2 Classical theory of gelation 103
3.3 Gelation in binary mixtures 114
3.A Moments of the Stockmayer distribution function 121
3.B Cascade theory of gelation 122
References 127
4 Elasticity of polymer networks 128
4.1 Thermodynamics of rubber elasticity 128
4.2 Affine network theory 133
4.3 Phantomnetwork theory 142
4.4 Swelling experiments 146
4.5 Volume transition of gels 150
4.6 Networks made up of nonlinear chains 156
References 159
5 Associating polymer solutions and thermoreversible gelation 160
5.1 Historical survey of the study of associating solutions 160
5.2 Statistical thermodynamics of associating polymers 161
5.3 Renormalization of the interaction parameters 168
5.4 Phase separation, stability limit, and other solution properties 169
5.5 Scattering function of associating polymer mixtures 170
5.A Renormalization of the interaction parameters 173
5.B Scattering function in RPA 175
5.C Spinodal condition in RPA 177
References 178
6 Nongelling associating polymers 180
6.1 Dimer formation as associated block-copolymers 180
6.2 Linear association and ring formation 186
6.3 Side-chain association 189
6.4 Hydration in aqueous polymer solutions and closed-loop miscibility gaps 197
6.5 Cooperative hydration in solutions of temperature-responsive polymers 200
6.6 Hydrogen-bonded liquid-crystalline supramolecules 207
6.7 Polymeric micellization 212
References 219
7 Thermoreversible gelation 222
7.1 Models of thermoreversible gelation 222
7.2 Application of the classical theory of gelation 224
7.3 Thermodynamics of sol–gel transition as compared with Bose–Einstein condensation 233
7.4 Thermoreversible gels with multiple cross-linking 235
References 245
8 Structure of polymer networks 247
8.1 Local structure of the networks–cross-linking regions 247
8.2 Global structure of the networks – elastically effective chains and elastic modulus 250
8.3 Percolation model 262
8.4 Self-similarity and scaling laws 269
8.5 Percolation in continuumm edia 276
References 279
9 Rheology of thermoreversible gels 281
9.1 Networks with temporal junctions 281
9.2 Linear response of transient networks 292
9.3 Stationary flows 299
9.4 Time-dependent flows 309
9.A Expansion in powers of the shear rate and time 321
9.B Solvable model of the quadratic dissociation rate 322
References 329
10 Some important thermoreversible gels 331
10.1 Polymer–surfactant interaction 331
10.2 Loop-bridge transition 339
10.3 Competing hydration and gelation 345
10.4 Coexisting hydration and gelation 352
10.5 Thermoreversible gelation driven by polymer conformational change 359
10.6 Thermoreversible gelation driven by the coil–helix transition of polymers 370
References 379
Index 383

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