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shijinwen金虫 (小有名气)
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[交流]
讨论一下“机械催化”产氢吧
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Domen Kazunari于1998年在CC上以“Mechano-catalytic overall water splitting”为题目，提出了全新的“机械催化产氢”的概念。之后，发表了一系列相关文章。 [98]Mechano-catalytic overall water splitting[Chem. Commun.] [99]Mechano-catalysis—a novel method for overall water splitting[PCCP] [00]A study of mechano-catalysts for overall water[JPCB] [00]Mechano-catalytic overall water splitting (II) nafion-deposited Cu2O[Applied Catalysis A：General] [00]Mechano-catalytic overall water splitting on some mixed oxides[Catalysis Today] [00]Mechano-catalytic overall water splitting on some oxides (II)[Applied Catalysis A：General] [00]Mechano-catalytic overall water-splitting into hydrogen and oxygen on some metal oxides[Applied Energy] 很多同行也对其提出了质疑。 [04]Comment on “A Study of Mechano-Catalysis for Overall Water Splitting”[JPCB] 请问各位对“机械催化产氢”或“机械催化”是怎么认识的？ [ Last edited by nxl5096224 on 2007-6-5 at 23:35 ] |
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shijinwen
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呵呵，文章中本身也提到了一些不能解释的问题 “As a whole, the experimental results in this work indicate the possibility of the redox mechanism for mechano-catalytic overall water splitting, but there exist several facts to be answered before the model is accepted.” 个人以为，文章中的实验现象有讨论价值。姑且先抛开“机械催化”的概念的正确性，至少有一点需要我们解决：实验中遇到的反应的本质到底是什么？ |
18楼2006-12-06 22:33:48
daiqiguang
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2楼2006-12-05 18:16:27
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3楼2006-12-05 18:55:11
daiqiguang
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文章还挺多的 A note on the gas-evolution of mechano-catalytic water-splitting system • SHORT COMMUNICATION International Journal of Hydrogen Energy, Volume 26, Issue 4, April 2001, Page 401 T. Ohta Mechano-catalytic overall water splitting on some mixed oxides • ARTICLE Catalysis Today, Volume 63, Issues 2-4, 25 December 2000, Pages 175-181 Go Hitoki, Tsuyosi Takata, Shigeru Ikeda, Michikazu Hara, Junko N. Kondo, Masato Kakihana and Kazunari Domen Efficiency of mechano-catalytic water-splitting system • ARTICLE International Journal of Hydrogen Energy, Volume 25, Issue 12, December 2000, Pages 1151-1156 T. Ohta On the theory of mechano-catalytic water-splitting system • ARTICLE International Journal of Hydrogen Energy, Volume 25, Issue 10, 1 October 2000, Pages 911-917 Tokio Ohta Energy systems and adaptive complexity • ARTICLE Applied Energy, Volume 67, Issues 1-2, September 2000, Pages 3-16 Tokio Ohta Mechano-catalytic overall water-splitting into hydrogen and oxygen on some metal oxides • ARTICLE Applied Energy, Volume 67, Issues 1-2, September 2000, Pages 159-179 Kazunari Domen, Shigeru Ikeda, Tsuyoshi Takata, Akira Tanaka, Michikazu Hara and Junko N. Kondo Mechano-catalytic water-splitting • ARTICLE Applied Energy, Volume 67, Issues 1-2, September 2000, Pages 181-193 Tokio Ohta Mechano-catalytic overall water splitting on some oxides (II) • ARTICLE Applied Catalysis A: General, Volume 200, Issues 1-2, 28 August 2000, Pages 255-262 Tsuyosi Takata, Shigeru Ikeda, Akira Tanaka, Michikazu Hara, Junko N. Kondo and Kazunari Domen Preliminary theory of mechano-catalytic water-splitting • ARTICLE International Journal of Hydrogen Energy, Volume 25, Issue 4, 1 April 2000, Pages 287-293 T. Ohta Mechano-catalytic overall water splitting (II) nafion-deposited Cu2O • ARTICLE Applied Catalysis A: General, Volume 190, Issues 1-2, 3 January 2000, Pages 35-42 Michikazu Hara, Hironori Hasei, Masaaki Yashima, Sigeru Ikeda, Tsuyoshi Takata, Junko N. Kondo and Kazunari Domen 发两篇大家共同研究 |
5楼2006-12-05 19:32:00