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小木虫论坛-学术科研互动平台 » 化学化工区 » 催化 » 催化反应 » 讨论一下“机械催化”产氢吧
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shijinwen

金虫 (小有名气)

[交流] 讨论一下“机械催化”产氢吧

Domen Kazunari于1998年在CC上以“Mechano-catalytic overall water splitting”为题目，提出了全新的“机械催化产氢”的概念。之后，发表了一系列相关文章。
[98]Mechano-catalytic overall water splitting[Chem. Commun.]
[99]Mechano-catalysis—a novel method for overall water splitting[PCCP]
[00]A study of mechano-catalysts for overall water[JPCB]
[00]Mechano-catalytic overall water splitting (II) nafion-deposited Cu2O[Applied Catalysis A：General]
[00]Mechano-catalytic overall water splitting on some mixed oxides[Catalysis Today]
[00]Mechano-catalytic overall water splitting on some oxides (II)[Applied Catalysis A：General]
[00]Mechano-catalytic overall water-splitting into hydrogen and oxygen on some metal oxides[Applied Energy]

很多同行也对其提出了质疑。
[04]Comment on “A Study of Mechano-Catalysis for
Overall Water Splitting”[JPCB]

请问各位对“机械催化产氢”或“机械催化”是怎么认识的？

[ Last edited by nxl5096224 on 2007-6-5 at 23:35 ]
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MCM Mobil Composite of Matter; SBA University of California Santa Barbara 光催化QQ群33982937
1楼 2006-12-05 17:08:25
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shijinwen

金虫 (小有名气)
引用回帖:
berlin(金币+3):Go on, Can U give U reason?

我认为传质作为控制步骤地可能性比较小。因为据文献中报道，CuO无活性，而Cu2O有活性，价态的变化会导致活性迥然的差异。如果说传质是控制步骤，那么我没法理解价态的变化和传质的联系。

[ Last edited by shijinwen on 2006-12-6 at 16:04 ]
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MCM Mobil Composite of Matter; SBA University of California Santa Barbara 光催化QQ群33982937
16楼2006-12-06 16:00:59
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daiqiguang

荣誉版主 (知名作家)

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机械催化???没听说过，看样子真是孤陋寡闻啊！！学习学习！！
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有事请到www.chemj.cn上找chemj，谢谢
2楼2006-12-05 18:16:27
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可可西里

木虫之王 (文学泰斗)

甾体者说
引用回帖:
Originally posted by daiqiguang at 2006-12-5 06:16 PM:
机械催化???没听说过，看样子真是孤陋寡闻啊！！学习学习！！

我是光催的

听过这个

感觉有点奇怪
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求助文献下载后，及时评分和EPI。
3楼2006-12-05 18:55:11
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daiqiguang

荣誉版主 (知名作家)

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引用回帖:
Originally posted by shijinwen at 2006-12-5 05:08 PM:
Domen Kazunari于1998年在CC上以“Mechano-catalytic overall water splitting”为题目，提出了全新的“机械催化产氢”的概念。之后，发表了一系列相关文章。
[98]Mechano-catalytic overall water splitting[Ch ...

文章还挺多的
A note on the gas-evolution of mechano-catalytic water-splitting system  • SHORT COMMUNICATION
International Journal of Hydrogen Energy, Volume 26, Issue 4, April 2001, Page 401 T. Ohta

        Mechano-catalytic overall water splitting on some mixed oxides  • ARTICLE
Catalysis Today, Volume 63, Issues 2-4, 25 December 2000, Pages 175-181
Go Hitoki, Tsuyosi Takata, Shigeru Ikeda, Michikazu Hara, Junko N. Kondo, Masato Kakihana and Kazunari Domen

        Efficiency of mechano-catalytic water-splitting system  • ARTICLE
International Journal of Hydrogen Energy, Volume 25, Issue 12, December 2000, Pages 1151-1156
T. Ohta

        On the theory of mechano-catalytic water-splitting system  • ARTICLE
International Journal of Hydrogen Energy, Volume 25, Issue 10, 1 October 2000, Pages 911-917
Tokio Ohta

        Energy systems and adaptive complexity  • ARTICLE
Applied Energy, Volume 67, Issues 1-2, September 2000, Pages 3-16
Tokio Ohta

        Mechano-catalytic overall water-splitting into hydrogen and oxygen on some metal oxides  • ARTICLE
Applied Energy, Volume 67, Issues 1-2, September 2000, Pages 159-179
Kazunari Domen, Shigeru Ikeda, Tsuyoshi Takata, Akira Tanaka, Michikazu Hara and Junko N. Kondo

        Mechano-catalytic water-splitting  • ARTICLE
Applied Energy, Volume 67, Issues 1-2, September 2000, Pages 181-193
Tokio Ohta

        Mechano-catalytic overall water splitting on some oxides (II)  • ARTICLE
Applied Catalysis A: General, Volume 200, Issues 1-2, 28 August 2000, Pages 255-262
Tsuyosi Takata, Shigeru Ikeda, Akira Tanaka, Michikazu Hara, Junko N. Kondo and Kazunari Domen

        Preliminary theory of mechano-catalytic water-splitting  • ARTICLE
International Journal of Hydrogen Energy, Volume 25, Issue 4, 1 April 2000, Pages 287-293
T. Ohta

        Mechano-catalytic overall water splitting (II) nafion-deposited Cu2O  • ARTICLE
Applied Catalysis A: General, Volume 190, Issues 1-2, 3 January 2000, Pages 35-42
Michikazu Hara, Hironori Hasei, Masaaki Yashima, Sigeru Ikeda, Tsuyoshi Takata, Junko N. Kondo and Kazunari Domen

发两篇大家共同研究
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5楼2006-12-05 19:32:00
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