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[交流] Molecules特刊邀稿专题-CO2催化转化利用

Molecules特刊邀稿专题-CO2催化转化利用

Molecules 杂志特刊 (ISSN 1420-3049), IF: 2.861
投稿截止日期: 2019年12月31日


特刊客邀编辑

客邀主编
Dr. Hamidreza Arandiyan
悉尼大学,化学学院,可持续发展先进催化实验室,澳大利亚
个人网址 https://sydney.edu.au/science/people/hamid.arandiyan.php  | 邮箱链接 hamid.arandiyan@sydney.edu.au
研究方向:钙钛矿型氧化物;多相催化;纳米材料;金属氧化物;纳米催化;大孔介孔材料;CO2的捕获和利用

客邀副主编
Yuan Wang(王媛)
新南威尔士大学,化学工程系,纳米粒子与催化研究组,澳大利亚
个人网址 | 邮箱链接
研究方向:二氧化碳还原;环境催化;多孔纳米催化剂;能源催化转化与利用

各位专家学者,

后工业革命正面临两大挑战,即能源危机和全球变暖。将二氧化碳加氢制成燃料(闭合碳循环回路)为可再生能源提供能源储存解决方案,成为当前能源短缺和可持续发展问题的可行性技术。尽管学者在CO2甲烷化方面已经做出了很多努力,但由于这个反应是一个能源密集型工艺且需要高温条件,有效激活热力学稳定的CO2分子仍然是一个挑战。
H2催化还原CO2可通过多种反应产生不同的产物,例如通过反向水煤气变换(RWGS)反应产生CO,通过选择性加氢产生甲醇以及结合CO2还原和费托反应产氢。对这些路线的研究表明,反应中间体的稳定化对于控制催化剂选择性至关重要。众所周知,负载在各种氧化物(例如,Al2O3,TiO2,SiO2,CeO2和ZrO2)上的贵金属,例如Pt,Rh和Ru在相对温和的操作条件下可以催化CO2还原,然而它们的高成本限制了其实际应用。

此特刊欢迎学者积极投稿相关文章,包括催化剂失活和中毒,微波/超声波/等离子体辅助催化,高通量实验,机理研究,新型反应介质(超临界溶剂,离子液体等)在内的多相催化的各个领域的研究论文,以及催化剂的制备和改性,反应动力学研究,光谱表征,表面科学,理论和建模,传输效应(质量热)。针对二氧化碳还原反应的催化剂制备,例如双金属/合金催化剂,胶体催化剂,介孔材料,金属催化剂(固体,载体),金属氧化物,自组装催化剂,溶胶-凝胶催化剂,沸石,钙钛矿,尖晶石等。

Hamidreza Arandiyan博士
Yuan Wang (王媛)
访客编辑



关键词
1.能源材料;
2.二氧化碳转化;
3.微波/超声波/等离子体辅助催化;
4.催化剂的失活和中毒;
5.催化剂的制备和改性;
6.光谱表征;
7.表面科学;
8.双金属/合金催化剂;
9.钙钛矿混合氧化物催化剂;
10.过渡金属氧化物催化剂;

Special Issue "Converting CO2 into Fuel and Chemicals"

A special issue of Molecules (ISSN 1420-3049), IF: 2.861.
Deadline for manuscript submissions: 31 December 2019

Special Issue Editor


Guest Editor
Dr. Hamidreza Arandiyan
Laboratory of Advanced Catalysis for Sustainability, School of Chemistry, The University of Sydney, Sydney 2006, Australia
Website | E-Mail
Interests: Perovskite-type oxides; heterogeneous catalysis; nanomaterial design, rational design of metal oxides; nanocatalysis; mesoporous materials; CO2 reduction.

Guest Editor
Yuan Wang
Particles and Catalysis Research Group, School of Chemical Engineering, The University of New South Wales, Sydney 2052, Australia
Website | E-Mail
Interests: Carbon dioxide reduction; environmental catalysis; porous materials; nano-materials; energy-related applications.

Dear Colleagues,

The post-industrial revolution world is facing two major challenges, namely an energy crisis and global warming. The hydrogenation of exhausted CO2 to fuel (closing the loop of carbon recycling) provides an energy storage solution for intermittent renewable sources, which can be then used as fuel or feedstock for consumer products; therefore becoming a viable technological solution to current energy shortage and sustainability issues. Although many efforts have been made in relation to catalytic CO2 methanation, effectively activating the thermodynamically stable CO2 molecule continues to be an obstacle as it requires high temperatures and is an energy-intensive process.
The catalytic reduction of CO2 by H2 can lead to the formation of several types of products, such as CO produced through the reverse water–gas shift (RWGS) reaction, methanol generated via selective hydrogenation, and hydrocarbons formed through combination of CO2 reduction with Fischer–Tropsch (FT) reactions. Investigations into these routes reveal that the stabilization of key reaction intermediates is critically important for controlling catalytic selectivity. Precious metals, such as Pt, Rh, and Ru, supported on various oxides (e.g. Al2O3, TiO2, SiO2, CeO2, and ZrO2) are well known to promote CO2 reduction under relatively mild operating conditions, however, their high cost, as well as limited availability, restricts their practical application.

Research articles in all areas of heterogeneous catalysis including deactivation and poisoning of catalysts, microwave/ultrasonic/plasma assisted catalysis, high throughput experimentation, mechanistic studies, new reaction media (supercritical solvents, ionic liquids, etc.), preparation and modification of catalysts, reaction kinetics and engineering aspects, spectroscopic characterization, surface science, theory and modelling, transport effects (heat of mass) from both experimental and computational perspectives are encouraged. Articles focusing on bimetallic/alloy catalysts, colloidal catalysts, mesoporous materials, metal catalysts (solid, supported or not), metal oxides, self-assembled catalysts, sol-gel catalysts, supported catalysts, zeolites, perovskite, spinel are welcome as well.

Dr. Hamidreza Arandiyan
Yuan Wang
Guest Editors


Keywords
1.        Energy materials;
2.        CO2 conversion;
3.        Microwave/ultrasonic/plasma assisted catalysis
4.        Deactivation and poisoning of catalysts
5.        Preparation and modification of catalysts
6.        Spectroscopic characterization
7.        Surface science
8.        Bimetallic/alloy catalysts
9.        Perovskite mixed oxide catalysts
10.        Transition metal oxide catalysts
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