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界面催化——Interfacial Catalysis
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ISBN: 0824708393 Title: Interfacial Catalysis Author: Alexander G. Volkov Publisher: CRC Publication Date: 2002-12-12 Number Of Pages: 680 Editorial Description A comprehensive volume on interfacial catalysis, this book includes contributions from an international group of specialists in chemistry, environmental science, informatics, physiology, nuclear energy, and physics. The editor has organized the material into the main topics of fundamental characteristics, phase transfer catalysis, reversed micelles, biological aspects, and interfacial photocatalysis. Individual topics include self-organized microheterogeneous structures, nanochemistry, interfaci ...read whole description Preface Interfacial catalysis plays a key role in many chemical, physical, and biological processes. The past decade has witnessed a huge increase of research interest in the study of interfacial catalysis at liquid interfaces. Processes taking place at the interface between two immiscible liquid phases are fundamental to life since virtually all energy conversion processes in living organisms occur at liquid interfaces. The properties of liquid–liquid interfaces are very important for a variety of industries, including biotechnology, organic synthesis, nanochemistry, catalysis, pharmaceuticals, cosmetics, paints, detergents, oil extraction processes, and mining. The interface between two immiscible liquids with immobilized photosynthetic pigments serves as a convenient model for investigating photoprocesses that are accompanied by spatial separation of charges. The efficiency of charge separation is defined by the quantum yield of any photochemical reaction. Heterogeneous systems in which the oxidants and the reductants are either in different phases or sterically separated are the most effective in this regard. Different solubilities of the substrates and reaction products in the two phases of heterogeneous systems can alter the redox potential of reactants, making it possible to carry out reactions that cannot be performed in a homogeneous phase. The book is organized into five parts. Part I consists of seven chapters and deals with fundamental aspects of interfacial phenomena such as catalytic properties of liquid interfaces, electrochemistry at polarized interfaces, ion solvation and resolvation, interfacial potentials, separations, and interfacial catalysis in metal complexation and in enhanced oil recovery. Part II contains four chapters about history, theory, molecular mechanisms, synthesis, and experimental systems in phase transfer catalysis. Part III deals with micellar catalysis, enzymology, and photochemical reactions in reversed micelles. The chapters in Part IV discuss biological aspects of interfacial and membrane catalysis including bioelectrocatalysis, ion channels, mechanisms of respiration and photosynthesis, membrane catalysis, and ion transport processes. Part V, which is about interfacial photocatalysis, includes such topics as nanochemistry, nanoparticles, self-organized microheterogeneous structures, photosensitizers, and photocatalytic oxygen evolution. The experimental systems and theoretical analysis of interfacial photocatalytic systems are also discussed in Chapters 14, 15, and 18. I would like to extend my thanks to the authors for the time they spent on this project and for teaching us about their work on nanochemistry and interfacial catalysis. I also thank our Acquisitions Editor, Anita Lekhwani, and our Production Editor, Joseph Stubenrauch, for their friendly and courteous assistance. Alexander G. Volkov Copyright © 2003 by Taylor & Francis Group, LLC Contents Preface Contributors Part I. Interfacial Phenomena 1. Interfacial Catalysis at Oil/Water Interfaces Alexander G. Volkov 2. Electrochemistry of Chemical Reactions at Polarized Liquid–Liquid Interfaces Takashi Kakiuchi 3. Interfacial Catalysis in Metal Complexation Hitoshi Watarai 4. The Role of Water Molecules in Ion Transfer at the Oil/Water Interface Toshiyuki Osakai 5. Interfacial Potential and Distribution Equilibria Between Two Immiscible Electrolyte Solutions Le Quoc Hung 6. Use of Cyclodextrins or Porous Inorganic Supports to Improve Organic/ Aqueous Interfacial Transfers Martine Urrutigo?¨ty and Philippe Kalck 7. Ultrathin Films: Their Use in Enhanced Oil Recovery and in Interfacial Catalysis Lu Zhang, Sui Zhao, Jia-Yong Yu, Angelica L. Ottova´, and H. Ti Tien Part II. Phase Transfer Catalysis 8. Phase Transfer Catalysis Mieczysiaw Ma?kosza and Michai Fedoryn´ski 9. Liquid–Liquid Phase Transfer Catalysis: Basic Principles and Synthetic Applications Domenico Albanese 10. Phase Transfer Catalysis: Fundamentals and Selected Systems Jing-Jer Jwo 11. Interfacial Mechanism and Kinetics of Phase-Transfer Catalysis Hung-Ming Yang and Ho-Shing Wu Part III. Micellar Catalysis 12. Enzymes in Reverse Micelles (Microemulsions): Theory and Practice Andrey V. Levashov and Natalia L. Klyachko 13. Micellar Catalysis Vincent C. Reinsborough 14. Multiple Effects of Water Pools and Their Interfaces Formed by Reversed Micelles on Enzymic Reactions and Photochemistry Ayako Goto, Yuko Ibuki, and Rensuke Goto Part IV. Interfacial Biocatalysis and Membrane Catalysis 15. Supported Planar BLMs (Lipid Bilayers): Formation, Methods of Study, and Applications Angelica L. Ottova´ and H. Ti Tien 16. Bioelectrocatalysis Kenji Kano and Tokuji Ikeda 17. Energetics and Gating of Narrow Ionic Channels: The Influence of Channel Architecture and Lipid–Channel Interactions Peter C. Jordan, Gennady V. Miloshevsky, and Michael B. Partenskii 18. Biocatalysis: Electrochemical Mechanisms of Respiration and Photosynthesis Alexander G. Volkov 19. New Types of Membrane Reactions Mimicking Biological Processes Sorin Kihara 20. Ion-Transport Processes Through Membranes of Various Types: Liquid Membrane, Thin Supported Liquid Membrane, and Bilayer Lipid Membrane Osamu Shirai and Sorin Kihara Part V. Interfacial Photocatalysis 21. Development of Structurally Organized Photocatalytic Systems for Photocatalytic Hydrogen Evolution on the Basis of Lipid Vesicles with Semiconductor Nanoparticles Fixed on Lipid Membranes Oxana V. Vassiltsova and Valentin N. Parmon 22. Catalysis and Photocatalysis at Polarized Molecular Interfaces: An Electrochemical Approach to Catalytic Processes Based on Two-Phase Systems, Self-Organized Microheterogeneous Structures, and Unsupported Nanoparticles Riikka Lahtinen, Henrik Jensen, and David J. Ferm?´n 23. Photosensitizers at Interfaces of Model Membranes Sarah A. Gerhardt and Jin Z. Zhang http://www.namipan.com/d/7591a9d31ac6fbf8942fe87dc414907be4ca2171f1a62800 http://www.namipan.com/d/347c20d30bd41c3f51d9ac0d4b8e1c727e3f9541c1533800 [ Last edited by a410731466 on 2009-2-2 at 08:39 ] |
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