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the CO production rate increases almost linearly up to illumination intensities of 50 mW·cm?2 (which corresponds to an incident photon flux of approximately 1.32 × 1017 photons·s?1). We observe that the CO production levels off with illumination intensities above this value, suggesting that the CO production rate is not limited by the light absorption past this point and that another step in the photoredox cycle is limiting the overall solar-to-fuel conversion efficiency . 发自小木虫Android客户端 |
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