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李灿院士在ACCOUNTS OF CHEMICAL RESEARCH（影响因子21.84） 发的最新关于光解水综述 已有31人参与
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国内光催化研究牛人之一李灿院士的又一篇顶尖综述，欢迎大家共同探讨光催化领域的前沿，大家一起努力！！！！ This Account describes the important roles of cocatalysts in photocatalytic and PEC water splitting reactions. For semiconductor-based photocatalytic and PEC systems, we show that loading proper cocatalysts, especially dual cocatalysts for reduction and oxidation, on semiconductors (as light harvesters) can significantly enhance the activities of photocatalytic and PEC water splitting reactions. Loading oxidation and/or reduction cocatalysts on semiconductors can facilitate oxidation and reduction reactions by providing the active sites/reaction sites while suppressing the charge recombination and reverse reactions. In a PEC water splitting system, the water oxidation and reduction reactions occur at opposite electrodes, so cocatalysts loaded on the electrode materials mainly act as active sites/reaction sites spatially separated as natural photosynthesis does. In both cases, the nature of the loaded cocatalysts and their interaction with the semiconductor through the interface/junction are important.[ Last edited by 0809293 on 2013-3-29 at 11:13 ] |
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