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Chem最新综述ransient Directing Groups for Transformative C–H
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Online Now Articles REVIEWSwitch to Standard View Transient Directing Groups for Transformative C–H Activation by Synergistic Metal Catalysis Parthasarathy Gandeepan, Lutz Ackermann'Correspondence information about the author Lutz AckermannEmail the author Lutz Ackermann Publication stage: In Press Corrected Proof Transient Directing Groups for Transformative C–H Activation by Synergistic Metal Catalysis DOI: http://dx.doi.org/10.1016/j.chempr.2017.11.002 showArticle Info PDF (2 MB) Download Images(.ppt) Email Article Add to My Reading List Export Citation Create Citation Alert Cited by in Scopus (0) Summary Full Text Images/Data References Related Articles Comments Graphical Abstract Figure thumbnail fx1 The Bigger Picture Transition-metal-catalyzed C–H activation enables the use of easily accessible feedstocks for molecular syntheses, which holds great potential for sustainable syntheses. These C–H functionalizations are largely achieved by proximity-induced reactivity, exploiting strongly coordinating directing groups to ensure the required positional selectivity in intermolecular transformations. Since the installation and removal of the strongly coordinating directing groups calls for additional reaction steps, undesired waste is formed, which compromises the overall step- and atom-economical nature of C–H activation technology. Further, performing C–H activations with weakly coordinating functional groups continues to represent a formidable challenge. In this review,  萨达.png |
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